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I don't know much about asphyxiation but it does not sound comfortable. Concerning lethal injection, it's not certain how much pain the paralyzed body feels as the heart is being stopped – have there been EEG studies?
I would prefer execution by firing squad.
It's supposed to be very painless. If I remember correctly your body can't tell the difference between oxygen and nitrogen so you don't have a feeling of lack of air, just continue breathing normally then fall asleep and expire.
Generally, the build up of CO2 is what triggers pain and panic of asphyxiation. Oxygen displacing gases certainly do cause fast unconsciousness and brain damage. Would seem very likely that nitrogen works well.