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FWIW, nitrogen asphyxiation is one of the methods that's preferred by advocates of assisted suicide. Done correctly--by which I mean in a way that doesn't allow a buildup of CO2 in your bloodstream--it's not only painless but gives you a mild high. The proper way to do it is with something like a BiPAP, where the air that's being piped in is pure nitrogen, and the CO2 is all being removed immediately so you aren't breathing it back in. Without a buildup of CO2 in your bloodstream, your brain doesn't recognize that you're suffocating.
Have you ever breathed in helium from a balloon and gotten lightheaded? It's about like that.
I'm in favor of the death penalty in very, very rare cases--and this is not one where I would support it--and this is one of the surest, least barbaric ways to execute someone.
Let's tighten this up a bit.
Inert gas asphyxiation is very much a great way to go, but it's basically symptomless until after you lose consciousness.
You don't get high. The "high" people get is when they are choked out. I'm not really sure on the mechanism of that, though. You don't get lightheaded. The lightheadedness is from the blood oxygen levels increasing.
This is why it's very dangerous to enter enclosed spaces. You simply don't know you're about to die until it's too late. Plus, people come in to try to rescue you and succumb as well.
Anyway, lots of people have this experience. It's a common part of training for rebreathers for use in scuba diving.
As far as good ways to die, inert gas asphyxiation is up there with "proper" lethal injection (i.e. with a commercial euthanasia drug), opiate overdose, or just anesthetizing the being and doing whatever gets the job done.
Nitrogen can cause a "high" (aka nitrogen narcosis), but this effect only occurs at high pressures. So it is only a practical concern for divers, because they have to breathe high pressure air. Some divers replace the nitrogen in their tanks with other gases to avoid it.
It is unrelated to asphyxiation, and can occur even when the lungs are properly exchanging oxygen and CO2. It is a poorly understood direct interaction between high pressure nitrogen and the brain that does not occur at atmospheric pressure.
When I did my deep diving certification one of the things they got us to do was try and do maths of varying complexity (compared to previously doing it on the surface). I didn’t feel high at all, but most of us had slower response times and more errors at depth, apparently as a side effect of the increased nitrogen. Pretty wild.